RESUMO

We have produced and characterized spin-squeezed states at a temperature of 26 °C in a nuclear magnetic resonance quadrupolar system. The experiment was carried out on 133Cs nuclei of spin I=7/2 in a sample of lyotropic liquid crystal. The source of spin squeezing was identified as the interaction between the quadrupole moment of the nuclei and the electric field gradients present within the molecules. We use the spin angular momentum representation to describe formally the nonlinear operators that produce the spin squeezing on a Hilbert space of dimension 2I+1=8. The quantitative and qualitative characterization of this spin-squeezing phenomenon is expressed by a squeezing parameter and squeezing angle developed for the two-mode Bose-Einstein condensate system, as well as by the Wigner quasiprobability distribution function. The generality of the present experimental scheme points to potential applications in solid-state physics.

RESUMO

We report the experimental measurement of bipartite quantum correlations of an unknown two-qubit state. Using a liquid state Nuclear Magnetic Resonance setup and employing geometric discord, we evaluate the quantum correlations of a state without resorting to prior knowledge of its density matrix. The method is applicable to any 2 ⊗ d system and provides, in terms of number of measurements required, an advantage over full state tomography scaling with the dimension d of the unmeasured subsystem. The negativity of quantumness is measured as well for reference. We also observe the phenomenon of sudden transition of quantum correlations when local phase and amplitude damping channels are applied to the state.

RESUMO

Nuclear magnetic resonance (NMR) was successfully employed to test several protocols and ideas in quantum information science. In most of these implementations, the existence of entanglement was ruled out. This fact introduced concerns and questions about the quantum nature of such bench tests. In this paper, we address some issues related to the non-classical aspects of NMR systems. We discuss some experiments where the quantum aspects of this system are supported by quantum correlations of separable states. Such quantumness, beyond the entanglement-separability paradigm, is revealed via a departure between the quantum and the classical versions of information theory. In this scenario, the concept of quantum discord seems to play an important role. We also present an experimental implementation of an analogue of the single-photon Mach-Zehnder interferometer employing two nuclear spins to encode the interferometric paths. This experiment illustrates how non-classical correlations of separable states may be used to simulate quantum dynamics. The results obtained are completely equivalent to the optical scenario, where entanglement (between two field modes) may be present.

RESUMO

Nonclassical correlations play a crucial role in the development of quantum information science. The recent discovery that nonclassical correlations can be present even in separable (nonentangled) states has broadened this scenario. This generalized quantum correlation has been increasing in relevance in several fields, among them quantum communication, quantum computation, quantum phase transitions, and biological systems. We demonstrate here the occurrence of the sudden-change phenomenon and immunity against some sources of noise for the quantum discord and its classical counterpart, in a room temperature nuclear magnetic resonance setup. The experiment is performed in a decohering environment causing loss of phase relations among the energy eigenstates and exchange of energy between system and environment, resulting in relaxation to the Gibbs ensemble.

RESUMO

The quantification of quantum correlations (other than entanglement) usually entails labored numerical optimization procedures also demanding quantum state tomographic methods. Thus it is interesting to have a laboratory friendly witness for the nature of correlations. In this Letter we report a direct experimental implementation of such a witness in a room temperature nuclear magnetic resonance system. In our experiment the nature of correlations is revealed by performing only few local magnetization measurements. We also compared the witness results with those for the symmetric quantum discord and we obtained a fairly good agreement.

RESUMO

In this paper we present a series of high-resolution zero-field NMR spectra of the polycrystalline intermetallic compound GdAl(2). The spectra were obtained with the sample at 4.2K in the ordered magnetic state and in the absence of an external static magnetic field. Using a sequence composed of two RF pulses, we obtained up to five multi-quantum echoes for the (27)Al nuclei, which were used to construct the zero-field NMR spectra. The spectra obtained from the FID observed after the second pulse and the even echoes exhibited higher resolution than the odd ones. In order to explain such behavior, we propose a model in which there are two regions inside the sample with different inhomogeneous spectral-line broadenings. Moreover, with the enhanced resolution from the FID signal, we were able to determine quadrupolar couplings with great precision directly from the respective spectra. These results were compared with those obtained from the quadrupolar oscillations of the echo signals, and showed good agreement. Similar data were also obtained from (155)Gd and (157)Gd nuclei.

Assuntos

Alumínio/química , Gadolínio/química , Espectroscopia de Ressonância Magnética/métodos , Algoritmos , Cristalização , Campos Eletromagnéticos , Isótopos , Radioisótopos

RESUMO

This paper presents a description of nuclear magnetic resonance (NMR) of quadrupolar systems using the Holstein-Primakoff (HP) formalism and its analogy with a Bose-Einstein condensate (BEC) system. Two nuclear spin systems constituted of quadrupolar nuclei I=3/2 ((23)Na) and I=7/2 ((133)Cs) in lyotropic liquid crystals were used for experimental demonstrations. Specifically, we derived the conditions necessary for accomplishing the analogy, executed the proper experiments, and compared with quantum mechanical prediction for a Bose system. The NMR description in the HP representation could be applied in the future as a workbench for BEC-like systems, where the statistical properties may be obtained using the intermediate statistic, first established by Gentile. The description can be applied for any quadrupolar systems, including new developed solid-state NMR GaAS nanodevices.

RESUMO

This article reports a relaxation study in an oriented system containing spin 3/2 nuclei using quantum state tomography (QST). The use of QST allowed evaluating the time evolution of all density matrix elements starting from several initial states. Using an appropriated treatment based on the Redfield theory, the relaxation rate of each density matrix element was measured and the reduced spectral densities that describe the system relaxation were determined. All the experimental data could be well described assuming pure quadrupolar relaxation and reduced spectral densities corresponding to a superposition of slow and fast motions. The data were also analyzed in the context of Quantum Information Processing, where the coherence loss of each qubit of the system was determined using the partial trace operation.

RESUMO

In this paper, we describe a quantum state tomography method based on global rotations of the spin system which, together with a coherence selection scheme, enables the complete density matrix reconstruction. The main advantage of this technique, in respect to previous proposals, is the use of much shorter rf pulses, which decreases significantly the time necessary for algorithm quantum state tomography. In this case, under adequate experimental conditions, the rf pulses correspond to simple spatial rotations of the spin states, and its analytical description is conveniently given in the irreducible tensor formalism. Simulated results show the feasibility of the method for a single spin 72 nucleus. As an experimental result, we exemplify the application of this method by tomographing the steps during the implementation of the Deutsch algorithm. The algorithm was implemented in a (23)Na quadrupole nucleus using the strongly modulated pulses technique. We also extended the tomography method for a 3-coupled homonuclear spin 12 system, where an additional evolution under the internal Hamiltonian is necessary for zero order coherences evaluation.