RESUMO
Neutron techniques to characterize materials have a wide range of applications, one of the major developments being the identification of terrorist threats with chemical, biological, radiological, nuclear and explosives (CBRNE) materials. In this work, a thermal neutron irradiation system, using a241Am/9Be source of 111 GBq inside polyethylene cylindrical moderators, has been designed, built and tested. The geometry of moderator and the neutron source position were fixed trying to maximize the thermal neutrons flux emitted from the system. Therefore, the system is in fact a thermalized neutron source taking advantage of the backscattered neutrons, achieving thermal fluence rates of up to 5.3x102â¯cm-2â¯s-1, with dominantly thermal spectra. Samples can be placed there for several hours and thereafter be measured to identify their component elements by NAA (Neutron Activation Analysis). Through Monte Carlo techniques employing the MCNP6 code (Pelowitz et al., 2014), four different configurations with polyethylene cylinders were simulated to choose the most adequate geometry. The theoretical model was then replicated in the neutronics hall of the Neutron Measurements Laboratory of the Energy Engineering Department of Universidad Politécnica de Madrid (LMN-UPM), carrying out experimental measurements using a BF3 neutron detector. A high agreement between MCNP6 results and the experimental values measured was observed. Consequently, the system developed could be employed in future laboratory experiments, both for the identification of trace substances by NAA and for the calibration of neutron detection equipment.
RESUMO
A thermal neutron system intended to be used in neutron activation analysis has been designed by Monte Carlo methods. The device is based on a241Am/9Be neutron source of 111 GBq, placed inside a cylindrical cavity open inside a parallelepiped of moderator material. Three different moderator materials, water, graphite and high-density polyethylene (HDPE), were simulated to check what is the most suitable for the detection system, concluding that HDPE reach the better performance. The device achieves an increased thermal neutron flux by taking advantage of neutron moderation in the polyethylene and the neutron scattering in the irradiation chamber walls. The thermal fluence rates obtained were 904â¯cm-2⯠s-1, i.e. 8.144â¯cm-2â¯s-1 GBq-1, with a fraction of thermal neutrons at the best point of 83% of pristine fast neutrons emitted by the source. The device has been designed by Monte Carlo techniques using the MCNP6 code, and the main tasks developed were to select the moderator material and to maximize the thermal neutrons flux in the irradiation chamber.